Nature of magnetic excitations in the iron pnictides and its pertinence to superconductivity as studied by inelastic neutron scattering

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2015-01-01
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Tucker, Gregory
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Robert J. McQueeney
Alan I. Goldman
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Physics and Astronomy
Physics and astronomy are basic natural sciences which attempt to describe and provide an understanding of both our world and our universe. Physics serves as the underpinning of many different disciplines including the other natural sciences and technological areas.
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Unconventional superconductivity and antiferromagnetism are often found in close proximity to one another. For the series of compounds Ba(Fe$_{1-x}$Co$_x$)$_2$As$_2$, which possesses both antiferromagnetism and superconductivity for the under-doped range of composition, this observation is certainly true. The close proximity, and in fact coexistence for under-doped Ba(Fe$_{1-x}$Co$_x$)$_2$As$_2$, of antiferromagnetism and superconductivity has encouraged speculation that antiferromagnetic spin fluctuations may mediate the electron pairing interaction in unconventional superconductors. Previous studies indicated that the spin fluctuations at optimally-doped Ba(Fe$_{1-x}$Co$_x$)$_2$As$_2$ are diffusive, while those at \bafeas are well defined spin wave excitations. Therefore, the nature of magnetic excitations in Ba(Fe$_{1-x}$Co$_x$)$_2$As$_2$ must change with the introduction of cobalt; but it is unclear if that change is merely a consequence of the loss of antiferromagnetic order, or a necessary ingredient for the appearance of superconductivity. To resolve this uncertainty, this work has been undertaken to study the spin fluctuations of five Ba(Fe$_{1-x}$Co$_x$)$_2$As$_2$ compositions varying in cobalt concentration from lightly-doped to nearly optimally-doped as well as representative samples of other, non-superconducting, transition metal substituted \bafeas compounds. The spin fluctuations of these samples, in their antiferromagnetically ordered and (where possible) superconducting states have been studied via triple-axis and time-of-flight inelastic neutron scattering, and definitively determine the importance of spin fluctuations for superconductivity in Ba(Fe$_{1-x}$Co$_x$)$_2$As$_2$.

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Thu Jan 01 00:00:00 UTC 2015