Competition between orthorhombic and re-entrant tetragonal phases in underdoped Ba1-xKxFe2As2 probed by the response to controlled disorder

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2019-02-26
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Timmons, Erik
Tanatar, Makariy
Willa, K.
Teknowijoyo, S.
Cho, Kyuil
Konczykowski, M.
Cavani, O.
Liu, Yong
Lograsso, Thomas
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Lograsso, Thomas
Ames Laboratory Division Director
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Physics and Astronomy
Physics and astronomy are basic natural sciences which attempt to describe and provide an understanding of both our world and our universe. Physics serves as the underpinning of many different disciplines including the other natural sciences and technological areas.
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Materials Science and Engineering
Materials engineers create new materials and improve existing materials. Everything is limited by the materials that are used to produce it. Materials engineers understand the relationship between the properties of a material and its internal structure — from the macro level down to the atomic level. The better the materials, the better the end result — it’s as simple as that.
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Ames National LaboratoryPhysics and AstronomyMaterials Science and Engineering
Abstract

Low-temperature (22 K) irradiation with 2.5-MeV electrons, creating point defects affecting elastic scattering, was used to study the competition between stripe C-2 and tetragonal C-4 antiferromagnetic phases which exist in a narrow doping range around x = 0.25 in hole-doped Ba1-xKxFe2As2. In nearby compositions outside of this range, at x = 0.22 and x = 0.19, the temperatures of both the concomitant orthorhombic/stripe antiferromagnetic transition T-C2 and the superconducting transition T-c are monotonically suppressed by added disorder at similar rates of about 0.1 K/mu Omega cm, as revealed through using resistivity variation as an intrinsic measure of scattering rate. In a stark contrast, a rapid suppression of the C-4 phase at the rate of 0.24 K/mu Omega cm is found at x = 0.25. Moreover, this suppression of the C-4 phase is accompanied by unusual disorder-induced stabilization of the C-2 phase, determined by resistivity and specific heat measurements. The rate of the C-4 phase suppression is notably higher than the suppression rate of the spin-vortex phase in the Ni-doped CaKFe4As4 (0.16 K/mu Omega cm).

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