Publication Date
1-18-2019
Department
Ames Laboratory; Physics and Astronomy
Campus Units
Physics and Astronomy, Ames Laboratory
OSTI ID+
1494937
Report Number
IS-J 9877
DOI
10.1103/PhysRevLett.122.027401
Journal Title
Physical Review Letters
Volume Number
122
Issue Number
2
First Page
027401
Abstract
Plasmonic metamaterials and metasurfaces offer new opportunities in developing high performance terahertz emitters and detectors beyond the limitations of conventional nonlinear materials. However, simple meta-atoms for second-order nonlinear applications encounter fundamental trade-offs in the necessary symmetry breaking and local-field enhancement due to radiation damping that is inherent to the operating resonant mode and cannot be controlled separately. Here we present a novel concept that eliminates this restriction obstructing the improvement of terahertz generation efficiency in nonlinear metasurfaces based on metallic nanoresonators. This is achieved by combining a resonant dark-state metasurface, which locally drives nonlinear nanoresonators in the near field, with a specific spatial symmetry that enables destructive interference of the radiating linear moments of the nanoresonators, and perfect absorption via simultaneous electric and magnetic critical coupling of the pump radiation to the dark mode. Our proposal allows eliminating linear radiation damping, while maintaining constructive interference and effective radiation of the nonlinear components. We numerically demonstrate a giant second-order nonlinear susceptibility ∼10−11 m/V, a one order improvement compared with the previously reported split-ring-resonator metasurface, and correspondingly, a 2 orders of magnitude enhanced terahertz energy extraction should be expected with our configuration under the same conditions. Our study offers a paradigm of high efficiency tunable nonlinear metadevices and paves the way to revolutionary terahertz technologies and optoelectronic nanocircuitry.
DOE Contract Number(s)
AC02-07CH11358; 320081; 61601166; 61701001; 61701003; 61722101; KJ2017ZD51; KJ2017ZD02
Language
en
Department of Energy Subject Categories
42 ENGINEERING
Publisher
Iowa State University Digital Repository, Ames IA (United States)
Included in
Engineering Physics Commons, Materials Science and Engineering Commons, Nanoscience and Nanotechnology Commons
