Spin dynamics in antiferromagnetic oxypnictides and fluoropnictides: LaMnAsO, LaMnSbO, and BaMnAsF

Thumbnail Image
Date
2020-04-15
Authors
Islam, Farhan
Gordon, Elijah
Das, Pinaki
Liu, Yong
Ke, Liquin
Abernathy, Douglas
McQueeney, Robert
Vaknin, David
Major Professor
Advisor
Committee Member
Journal Title
Journal ISSN
Volume Title
Publisher
Authors
Research Projects
Organizational Units
Organizational Unit
Organizational Unit
Physics and Astronomy
Physics and astronomy are basic natural sciences which attempt to describe and provide an understanding of both our world and our universe. Physics serves as the underpinning of many different disciplines including the other natural sciences and technological areas.
Journal Issue
Is Version Of
Versions
Series
Department
Ames National LaboratoryPhysics and Astronomy
Abstract

Inelastic neutron scattering (INS) from polycrystalline antiferromagnetic LaMnAsO, LaMnSbO, and BaMnAsF are analyzed using a J(1)-J(2)-J(c) Heisenberg model in the framework of the linear spin-wave theory. All three systems show clear evidence that the nearest- and next-nearest-neighbor interactions within the Mn square lattice layer (J(1) and J(2)) are both antiferromagnetic (AFM). However, for all compounds studied the competing interactions have a ratio of 2J(2)/J(1) < 1, which favors the square lattice checkerboard AFM structure over the stripe AFM structure. The interplane coupling Jc in all three systems is on the order of similar to 3 x 10(-4)J(1), rendering the magnetic properties of these systems with quasi-two-dimensional character. The substitution of Sb for As significantly lowers the in-plane exchange coupling, which is also reflected in the decrease of the Neel temperature, T-N. Although BaMnAsF shares the same MnAs sheets as LaMnAsO, their J(1) and J(2) values are substantially different. Using density functional theory, we calculate exchange parameters J(ij) to rationalize the differences among these systems.

Comments
Description
Keywords
Citation
DOI
Subject Categories
Copyright
Collections