Anomalous dynamical line shapes in a quantum magnet at finite temperature

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2012-01-01
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Tennant, D. A.
Lake, B.
James, A. J. A.
Essler, F. H. L.
Notbohm, S.
Mikeska, H.-J.
Fielden, J.
Kögerler, P.
Canfield, Paul
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Canfield, Paul
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Physics and Astronomy
Physics and astronomy are basic natural sciences which attempt to describe and provide an understanding of both our world and our universe. Physics serves as the underpinning of many different disciplines including the other natural sciences and technological areas.
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Ames National LaboratoryPhysics and Astronomy
Abstract

The effect of thermal fluctuations on the dynamics of a gapped quantum magnet is studied using inelastic neutron scattering on copper nitrate, a model material for the spin-1/2, one-dimensional (1D) bond alternating Heisenberg chain. A large, highly deuterated, single-crystal sample of copper nitrate is produced using a solution growth method and measurements are made using the high-resolution backscattering spectrometer OSIRIS at the ISIS Facility. Theoretical calculations and numerical analysis are combined to interpret the physical origin of the thermal effects observed in the magnetic spectra. The primary observations are (1) a thermally induced central peak due to intraband scattering, which is similar to Villain scattering familiar from soliton systems in 1D, and (2) the one-magnon quasiparticle pole is seen to develop with temperature into an asymmetric continuum of scattering. We relate this asymmetric line broadening to a thermal strongly correlated state caused by hard-core constraints and quasiparticle interactions. These findings are a counter example to recent assertions of the universality of line broadening in 1D systems and are applicable to a broad range of quantum systems.

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This article is published as Tennant, D. A., B. Lake, A. J. A. James, F. H. L. Essler, S. Notbohm, H-J. Mikeska, J. Fielden, P. Kögerler, P. C. Canfield, and M. T. F. Telling. "Anomalous dynamical line shapes in a quantum magnet at finite temperature." Physical Review B 85, no. 1 (2012): 014402. DOI: 10.1103/PhysRevB.85.014402. Posted with permission.

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Sun Jan 01 00:00:00 UTC 2012
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