Optical and magneto-optical properties of single crystals of RFe2 (R=Gd, Tb, Ho, and Lu) and GdCo2 intermetallic compounds

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1998
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Lee, Seong-Jae
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David W. Lynch
Paul C. Canfield
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Physics and Astronomy
Physics and astronomy are basic natural sciences which attempt to describe and provide an understanding of both our world and our universe. Physics serves as the underpinning of many different disciplines including the other natural sciences and technological areas.
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Abstract

We have studied the diagonal and off-diagonal optical conductivity of a RFe2(R=Gd, Tb, Ho, Lu) and GdCo2 single crystal grown by the flux method. Using spectroscopic ellipsometry we have measured the dielectric function from 1.5 to 5.5 eV. The magneto-optical parameters (Kerr rotation and ellipticity) were obtained using a magneto-optical polar Kerr spectrometer at temperatures between 7 and 295 K and applied magnetic fields between 0.5 to 1.6 T. The apparatus and calibration method are described in detail. Using magneto-optical data and optical constants we derive the experimental value of the off-diagonal conductivity components.;Theoretical calculations of optical conductivities and magneto-optical parameters were performed using the tight binding-linear muffin tin orbitals method within the local spin density approximation. We applied this TB-LMTO method to LuFe2. The obtained theoretical results agree well with the experimental data. The oxidation effects on the diagonal part of the optical conductivity were considered using a three phase model. The oxidation effects on the magneto-optical parameters were also considered by treating the oxide layer as a nonmagnetic thin transparent layer. These corrections change not only the magnitude but also the shape of the optical conductivity and the magneto-optical parameters.

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Thu Jan 01 00:00:00 UTC 1998