Magnetic x-ray scattering study of GdCo2Ge2 and NdCo2Ge2

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2002-01-01
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Good, William
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Physics and Astronomy
Physics and astronomy are basic natural sciences which attempt to describe and provide an understanding of both our world and our universe. Physics serves as the underpinning of many different disciplines including the other natural sciences and technological areas.
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In order to determine the interactions responsible for magnetic ordering in RCo2Ge2 compounds, where R is a rare earth element, it is necessary to obtain an accurate measurement of the wave vector and orientation of the moments. Resonant and nonresonant x-ray scattering experiments were performed in order to determine the magnetic structure of single crystal compounds of GdCo2Ge2 and NdC02Ge2. Both compounds order antiferromagnetically with a wave vector along the c-direction. GdCo2Ge2 orders in an incommensurate state characterized by a propagation wave vector [Tau] = (0 0 [Tau subscript z]). The value of [Tau subscript z] is temperature dependent and approaches 0.932(±0.002) r.l.u. below T[Subscript N]= 32.9 K. A peak corresponding to 3[Tau subscript z] was also observed at T= 6K. By comparison with theoretical cross sections, a Q dependent measurement indicates that the moments are aligned perpendicular to the c-axis. Susceptibility measurements on NdCo2Ge2 indicate that two transitions may occur at low temperature. An incommensurate structure was found with a wave vector (0 0 [Tau subscript z]) and [Tau subscript z]= 0.7420(±0.0003) r.l.u. An extensive search was carried out for a second transition, but no second phase was detected.

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Tue Jan 01 00:00:00 UTC 2002